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Drichko, Natalia ; Sugiura, Shiori ; Yamashita, Minoru ; Ueda, Akira ; Uji, Shinya ; Hassan, Nora ; Sunairi, Yoshiya ; Mori, Hatsumi ; Zhilyaeva, Elena I. ; Torunova, Svetlana ; et al ( , Physical Review B)
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Hassan, Nora M. ; Thirunavukkuarasu, Komalavalli ; Lu, Zhengguang ; Smirnov, Dmitry ; Zhilyaeva, Elena I. ; Torunova, Svetlana ; Lyubovskaya, Rimma N. ; Drichko, Natalia ( , npj Quantum Materials)
Abstract Strong electronic interactions can drive a system into a state with a symmetry breaking. Lattice frustration or competing interactions tend to prevent symmetry breaking, leading to quantum disordered phases. In spin systems frustration can produce a spin liquid state. Frustration of a charge degree of freedom also can result in various exotic states, however, experimental data on these effects is scarce. In this work we demonstrate how in a Mott insulator on a weakly anisotropic triangular lattice a charge ordered state melts on cooling down to low temperatures. Raman scattering spectroscopy finds that
-(BEDT-TTF)$$\kappa$$ Hg(SCN)$${}_{2}$$ Cl enters an insulating “dipole solid” state at$${}_{2}$$ , but below$$T=30\,{\mathrm{K}}$$ the order melts, while preserving the insulating energy gap. Based on these observations, we suggest a phase diagram relevant to other quantum paraelectric materials.$$T=15\,{\mathrm{K}}$$ -
Hassan, Nora ; Cunningham, Streit ; Mourigal, Martin ; Zhilyaeva, Elena I. ; Torunova, Svetlana A. ; Lyubovskaya, Rimma N. ; Schlueter, John A. ; Drichko, Natalia ( , Science)